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Portman appeared in the video for Banhart’s song "Carmensita." They were "just too different" to make it work, sources say.
She has been dating Brazilian actor Rodrigo Santoro for about a month according to In Touch Weekly.
However, Natalie turned down the offer because she wanted to concentrate on dancing and acting.
At the age of 13, Natalie Portman auditioned for the role of the young girl in Léon and got the role, starring in the film alongside Jean Reno and Gary Oldman.
The filming of Star Wars Episode II: Attack of the Clones took place in Portman's summer holiday in 2000.
The next year, she starred alongside Meryl Streep, Kevin Kline and Philip Seymour Hoffman in a New York City Public Theatre production of Chekhov's The Seagull.
Personal Life: Natalie Portman has been romantically linked with a number of male actors, including Jake Gyllenhaal, Gael Garcia Bernal and the musician Adam Levine.